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Tracing the impact of stack configuration on interface resistances in reverse electrodialysis by in situelectrochemical impedance spectroscopy

Frontiers of Environmental Science & Engineering 2022, Volume 16, Issue 4, doi: 10.1007/s11783-021-1480-9

Abstract:

• RED performance and stack resistance were studied by EIS and LSV.

Keywords： Reverse electrodialysis     Electrochemical impedance spectroscopy     Concentration polarization     Spacer shadow    

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Spin polarization strategy to deploy proton resource over atomic-level metal sites for highly selective CO electrolysis

Frontiers of Chemical Science and Engineering 2022, Volume 16, Issue 12,   Pages 1772-1781 doi: 10.1007/s11705-022-2197-4

Abstract: Unlocking of the extremely inert C=O bond during electrochemical CO2 reduction demands subtle regulation on a key “resource”, protons, necessary for intermediate conversion but also readily trapped in water splitting, which is still challenging for developing efficient single-atom catalysts limited by their structural simplicity usually incompetent to handle this task. Incorporation of extra functional units should be viable. Herein, a proton deployment strategy is demonstrated via “atomic and nanostructured iron (A/N-Fe) pairs”, comprising atomically dispersed iron active centers spin-polarized by nanostructured iron carbide ferromagnets, to boost the critical protonation steps. The as-designed catalyst displays a broad window (300 mV) for CO selectivity > 90% (98% maximum), even outperforming numerous cutting-edge M–N–C systems. The well-placed control of proton dynamics by A/N-Fe can promote *COOH/*CO formation and simultaneously suppress H2 evolution, benefiting from the magnetic-proximity-induced exchange splitting (spin polarization) that properly adjusts energy levels of the Fe sites’ d-shells, and further those of the adsorbed intermediates’ antibonding molecular orbitals.

Keywords： CO2 electrolysis     single-atom catalysts     spin polarization     proton dynamics     in situ IR spectroscopy     kinetic isotope effect    

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Development and application of ex-situ presulfurization technology for hydrotreating catalysts in China

Yulan GAO, Xiangchen FANG, Zhenmin CHENG

Frontiers of Chemical Science and Engineering 2011, Volume 5, Issue 3,   Pages 287-296 doi: 10.1007/s11705-010-0529-2

Abstract: The development and application of ex-situ presulfurization (EPRES) technology for hydrotreating catalysts

Keywords： ex-situ presulfurization     in situ presulfurization     hydrotreating catalyst     sulfur utilization ratio    

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Factors influencing near infrared spectroscopy analysis of agro-products: a review

Xiao XU, Lijuan XIE, Yibin YING

Frontiers of Agricultural Science and Engineering 2019, Volume 6, Issue 2,   Pages 105-115 doi: 10.15302/J-FASE-2019255

Abstract:

The near infrared (NIR) spectroscopy technique has wide applications in agriculture with the advantages

Keywords： agro-product     error source     influence factor     near infrared spectroscopy    

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Review: Tip-based vibrational spectroscopy for nanoscale analysis of emerging energy materials

Amun JARZEMBSKI, Cedric SHASKEY, Keunhan PARK

Frontiers in Energy 2018, Volume 12, Issue 1,   Pages 43-71 doi: 10.1007/s11708-018-0524-8

Abstract: Vibrational spectroscopy is one of the key instrumentations that provide non-invasive investigation ofHowever, diffraction of light fundamentally limits the spatial resolution of far-field vibrational spectroscopythis article, we thoroughly review the integration of atomic force microscopy (AFM) with vibrational spectroscopyFor example, photothermal induced resonance (PTIR) spectroscopy methods measure a sample’s local thermalsuccessfully breech the diffraction limit of light to provide nanoscale spatial resolution of vibrational spectroscopy

Keywords： vibrational spectroscopy     atomic force microscopy     photo-thermal induced resonance     scanning near-fieldoptical microscopy     tip-enhanced Raman spectroscopy     photo-induced force microscopy     molecular resonances    

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Terahertz time-domain spectroscopy of high-pressure flames

Jason BASSI, Mark STRINGER, Bob MILES, Yang ZHANG

Frontiers in Energy 2009, Volume 3, Issue 2,   Pages 123-133 doi: 10.1007/s11708-009-0033-x

Abstract: Laser spectroscopy in the visible and near infrared is widely used as a diagnostic tool for combustion

Keywords： terahertz time-domain spectroscopy     high-pressure flames     H2O absorption lines    

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Modeling of oil near-infrared spectroscopy based on similarity and transfer learning algorithm

Yifei Wang, Kai Wang, Zhao Zhou, Wenli Du

Frontiers of Chemical Science and Engineering 2019, Volume 13, Issue 3,   Pages 599-607 doi: 10.1007/s11705-019-1807-2

Abstract: Near-infrared spectroscopy mainly reflects the frequency-doubled and total-frequency absorption informationIn order to achieve rapid modeling of near-infrared spectroscopy and based on historical data of different

Keywords： near-infrared spectroscopy     transfer learning     similarity     modeling    

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Controlling the Reconstruction of Ni/CeO2 Catalyst during Reduction for Enhanced CO Methanation Article

Xinyu Cao,Tiancheng Pu,Bar Mosevitzky Lis,Israel E. Wachs,Chong Peng,Minghui Zhu,Yongkang Hu,

Engineering 2022, Volume 14, Issue 7,   Pages 94-99 doi: 10.1016/j.eng.2021.08.023

Abstract:

Reductive pretreatment is an important step for activating supported metal catalysts but has received little attention. In this study, reconstruction of the supported nickel catalyst was found to be sensitive to pretreatment conditions. In contrast to the traditional activation procedure in hydrogen, activating the catalyst in syngas created supported Ni nanoparticles with a polycrystalline structure containing an abundance of grain boundaries. The unique post-activation catalyst structure offered enhanced CO adsorption and an improved CO methanation rate. The current strategy to tune the catalyst structure via manipulating the activation conditions can potentially guide the rational design of other supported metal catalysts.

Keywords： Nickel–ceria catalyst     Catalyst activation     Crystallinity     Methanation     In situ spectroscopy    

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Polyolefin-nanocomposites with special properties by in-situ polymerization

Walter Kaminsky

Frontiers of Chemical Science and Engineering 2018, Volume 12, Issue 3,   Pages 555-563 doi: 10.1007/s11705-018-1715-x

Abstract:

Exceptionally strong polyolefin nanocomposites are synthesized by in-situ polymerization using

Keywords： polyolefin nanocomposites     metallocenes     methylaluminoxane    

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Time of flight improved thermally grown oxide thickness measurement with terahertz spectroscopy

Frontiers of Mechanical Engineering 2022, Volume 17, Issue 4, doi: 10.1007/s11465-022-0705-3

Abstract: As a nondestructive testing technique, terahertz time-domain spectroscopy technology is commonly used

Keywords： thermal barrier coatings     thermally grown oxide     terahertz spectroscopy     time of flight    

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Cystine-assisted accumulation of gold nanoparticles on ZnO to construct a sensitive surface-enhanced Raman spectroscopy

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 1,   Pages 15-23 doi: 10.1007/s11705-022-2177-8

Abstract: Recently, various semiconductor/metal composites have been developed to fabricate surface-enhanced Raman spectroscopyprovided a promising method to fabricate sensitive semiconductor/noble metal-based surface-enhanced Raman spectroscopy

Keywords： biomineralization     cystine     semiconductor/metal composite     SERS detection     Raman detection    

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Propagation characteristics of transient waves in low-strain integrity testing on cast-in-situ concrete

Hanlong LIU, Xuanming DING

Frontiers of Structural and Civil Engineering 2009, Volume 3, Issue 2,   Pages 240-240 doi: 10.1007/s11709-009-0100-8

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Thermodynamic analysis of liquid phase in situ hydrogenation of glycerol for 1,3-propanediol synthesis

Kun OUYANG, Yu HUANG, Haoyi CHEN, Tao LI, Fahai CAO, Dingye FANG

Frontiers of Chemical Science and Engineering 2011, Volume 5, Issue 1,   Pages 67-73 doi: 10.1007/s11705-010-0541-6

Abstract: reforming (APR) and catalytic hydrogenation of glycerol, a novel reaction system of liquid phase in situreforming reaction; the hydrogen generated from the APR of glycerol can be quickly transformed to the in situ

Keywords： glycerol     aqueous-phase reforming     1     3-propanediol     in-situ reduction    

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In situ-based assessment of soil liquefaction potential–Case study of an earth dam in Tunisia

Ikram GUETTAYA,Mohamed Ridha EL OUNI

Frontiers of Structural and Civil Engineering 2014, Volume 8, Issue 4,   Pages 456-461 doi: 10.1007/s11709-014-0259-5

Abstract: The present paper examines the evaluation of liquefaction potential of an earth dam foundation in Tunisia. The assessment of soil liquefaction was made using deterministic and probabilistic simplified procedures developed from several case histories. The data collected from the field investigation performed before and after the vibrocompaction are analyzed and the results are reported. The obtained results show that after vibrocompaction, a significant improvement of the soil resistance reduces the liquefaction potential of the sandy foundation. Indeed, in the untreated layers, the factor of safety drops below 1 which means that the soil is susceptible for liquefaction. However, in the compacted horizons, the values of exceed the unit which justifies the absence of liquefaction hazard of the foundation.

Keywords： liquefaction     cone penetration test (CPT)     standard penetration test (SPT)     vibrcompaction     sand    

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In situ synthesis of FeS/Carbon fibers for the effective removal of Cr(VI) in aqueous solution

Rongrong Zhang, Daohao Li, Jin Sun, Yuqian Cui, Yuanyuan Sun

Frontiers of Environmental Science & Engineering 2020, Volume 14, Issue 4, doi: 10.1007/s11783-020-1247-8

Abstract: Abstract • FeS/carbon fibers were in situ synthesized with Fe-carrageenan hydrogel fiber. • The doubleTherefore, this study investigates in situ synthesized FeS/carbon fibers with an Fe-carrageenan biomass

Keywords： Carrageenan     FeS     Double-helix structure     Hexavalent chromium    

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Title Author Date Type Operation

Tracing the impact of stack configuration on interface resistances in reverse electrodialysis by in situelectrochemical impedance spectroscopy

Journal Article

Spin polarization strategy to deploy proton resource over atomic-level metal sites for highly selective CO electrolysis

Journal Article

Development and application of ex-situ presulfurization technology for hydrotreating catalysts in China

Yulan GAO, Xiangchen FANG, Zhenmin CHENG

Journal Article

Factors influencing near infrared spectroscopy analysis of agro-products: a review

Xiao XU, Lijuan XIE, Yibin YING

Journal Article

Review: Tip-based vibrational spectroscopy for nanoscale analysis of emerging energy materials

Amun JARZEMBSKI, Cedric SHASKEY, Keunhan PARK

Journal Article

Terahertz time-domain spectroscopy of high-pressure flames

Jason BASSI, Mark STRINGER, Bob MILES, Yang ZHANG

Journal Article

Modeling of oil near-infrared spectroscopy based on similarity and transfer learning algorithm

Yifei Wang, Kai Wang, Zhao Zhou, Wenli Du

Journal Article

Controlling the Reconstruction of Ni/CeO2 Catalyst during Reduction for Enhanced CO Methanation

Xinyu Cao,Tiancheng Pu,Bar Mosevitzky Lis,Israel E. Wachs,Chong Peng,Minghui Zhu,Yongkang Hu,

Journal Article

Polyolefin-nanocomposites with special properties by in-situ polymerization

Walter Kaminsky

Journal Article

Time of flight improved thermally grown oxide thickness measurement with terahertz spectroscopy

Journal Article

Cystine-assisted accumulation of gold nanoparticles on ZnO to construct a sensitive surface-enhanced Raman spectroscopy

Journal Article

Propagation characteristics of transient waves in low-strain integrity testing on cast-in-situ concrete

Hanlong LIU, Xuanming DING

Journal Article

Thermodynamic analysis of liquid phase in situ hydrogenation of glycerol for 1,3-propanediol synthesis

Kun OUYANG, Yu HUANG, Haoyi CHEN, Tao LI, Fahai CAO, Dingye FANG

Journal Article

In situ-based assessment of soil liquefaction potential–Case study of an earth dam in Tunisia

Ikram GUETTAYA,Mohamed Ridha EL OUNI

Journal Article

In situ synthesis of FeS/Carbon fibers for the effective removal of Cr(VI) in aqueous solution

Rongrong Zhang, Daohao Li, Jin Sun, Yuqian Cui, Yuanyuan Sun

Journal Article